Search results for "phonon scattering"
showing 10 items of 35 documents
Thickness dependence of anomalous Hall conductivity in L10-FePt thin film
2019
L10 ordered alloys are ideal models for studying the anomalous Hall effect (AHE), which can be used to distinguish the origin from intrinsic (from band structure) or from extrinsic effects (from impurity scatterings). In the bulk limit of L10 ordered FePt films, the AHE is considered to be dominated by the intrinsic contribution, which mainly comes from the strong spin-orbit interaction (SOI) of Pt atoms and exchange-splitting of Fe atoms. The study of anomalous Hall conductivity (AHC) of L10-FePt thin films is of particular interest for its application in spintronic devices. In order to reduce the effects of defects such as grain boundaries, we chose SrTiO3 as the substrate which has a ver…
Existence of two time scales in the phase transitions of BaTiO3
1991
Abstract We report new Raman scattering measurements in the tetragonal phase of a single domain BaTiO3 crystal. Data reveal the occurence of a large quasi elastic scattering. The Raman profile is analysed in terms of coexisting soft phonon and Debye relaxation.
Nanowires: A route to efficient thermoelectric devices
2019
Miniaturization of electronic devices aims at manufacturing ever smaller products, from mesoscopic to nanoscopic sizes. This trend is challenging because the increased levels of dissipated power demands a better understanding of heat transport in small volumes. A significant amount of the consumed energy in electronics is transformed into heat and dissipated to the environment. Thermoelectric materials offer the possibility to harness dissipated energy and make devices less energy-demanding. Heat-to-electricity conversion requires materials with a strongly suppressed thermal conductivity but still high electronic conduction. Nanowires can meet nicely these two requirements because enhanced …
Low-temperature exciton absorption in InSe under pressure.
1992
We have investigated the effect of pressure on the lowest direct band-edge exciton of the layered semiconductor InSe by optical-absorption measurements at 10 K and for pressures up to 4 GPa. The Elliott-Toyozawa formalism is used to analyze the line shape of the exciton absorption spectra. In this way we determine the pressure dependence of the lowest direct band gap, the exciton binding energy, and the exciton linewidth. The band gap exhibits a pronounced nonlinear shift with pressure, which is a consequence of the strong anisotropy of intralayer and interlayer bonding. The exciton binding energy decreases with pressure, mainly due to the large increase of the low-frequency dielectric cons…
Phonon Scattering through a Local Anisotropic Structural Disorder in the Thermoelectric Solid Solution Cu_2Zn_(1−x)Fe_xGeSe_4
2013
Inspired by the promising thermoelectric properties of chalcopyrite-like quaternary chalcogenides, here we describe the synthesis and characterization of the solid solution Cu(2)Zn(1-x)Fe(x)GeSe(4). Upon substitution of Zn with the isoelectronic Fe, no charge carriers are introduced in these intrinsic semiconductors. However, a change in lattice parameters, expressed in an elongation of the c/a lattice parameter ratio with minimal change in unit cell volume, reveals the existence of a three-stage cation restructuring process of Cu, Zn, and Fe. The resulting local anisotropic structural disorder leads to phonon scattering not normally observed, resulting in an effective approach to reduce th…
Elastic light scattering from semiconductor structures: Localized versus propagating intermediate electronic excitations
1995
We present a theoretical study of the relative role of localized and propagating intermediate electronic states in the processes of elastic scattering of light. Only localized excitations lead to isotropic scattering in lowest-order perturbation theory. Inhomogeneous broadening of the optical transition affects the scattering efficiency from the ordered and disordered array of localized states in a qualitatively different way. The propagating electronic excitations may only contribute to elastic light scattering via higher-order processes. The scattering of excitons by impurities or the interface roughness potential is suggested as a mechanism for the contribution of propagating excitations…
A Composite Phononic Crystal Design for Quasiparticle Lifetime Enhancement in Kinetic Inductance Detectors
2019
A nanoscale phononic crystal filter (reflector) is designed for a kinetic inductance detector where the reflection band is matched to the quasiparticle recombination phonons with the aim to increase quasiparticle lifetime in the superconducting resonator. The inductor is enclosed by a 1 um wide phononic crystal membrane section with two simple hole patterns that each contain a partial spectral gap for various high frequency phonon modes. The phononic crystal is narrow enough for low frequency thermal phonons to propagate unimpeded. With 3D phonon scattering simulations over a 40 dB attenuation in transmitted power is found for the crystal, which was previously estimated to give a lifetime e…
<title>Raman scattering by phonons and magnons in Ni<formula><inf><roman>c</roman></inf></formula>Mg<for…
2003
ABSTRACT The Raman scattering by phonons and magnons was studied at room temperature in polycrystalline solid solutions NiMg1O and pure NiO. The experimental Raman spectrum of NiO consists of six well resolved bands, whose originis due to the disorder-induced one-phonon scattering (bands at 400 and 500 cm'), two-phonon scattering (bands at 750,900 and 1 100 cm) and two-magnon scattering (band at 1500 cm). In NiMg1O solid solutions, a relative increase ofone-phonon scattering is observed upon a dilution of nickel oxide by magnesium ions: at room temperature, the two-magnon band becomes invisible for c<O.7, whereas the two-phonon contribution disappears at c<O.5. Such behaviour isexplained by…
Proton-Hydrogen Charge Exchange and Elastic Scattering in the Faddeev Approach
2000
Results of the application of Faddeev-type integral equations to proton-hydrogen collisions are reported. The approach, realized in the impact parameter representation, incorporates the exact two-particle off-shell Coulomb T-matrices in all ‘triangle’ contributions to the effective potentials. Calculatedtotal and differential electron-transfer as well as differential elastic scattering cross sections show very good agreement with experiment, over a wide range of incident energies.
Fine tuning of thermoelectric performance in phase-separated half-Heusler compounds
2015
Two successful recipes to enhance the thermoelectric performance, namely carrier concentration optimization and reduction of thermal conductivity, have been combined and applied to the p-type (Ti/Zr/Hf)CoSb1−xSnx system. An intrinsic micrometer-scale phase separation increases the phonon scattering and reduces the lattice thermal conductivity. A substitution of 15% Sb by Sn optimizes the electronic properties. Starting from this, further improvement of the thermoelectric properties has been achieved by a fine tuning of the Ti to Hf ratio. The microstructuring of the samples was studied in detail with high-resolution synchrotron powder X-ray diffraction and element mapping electron microscop…